Jesse Kroll is playing a leading role in unraveling the extremely complex multiphase atmospheric chemistry of organic molecules emitted by both anthropogenic activities and biogenic processes. His work is particularly important because atmospheric organic species form a large fraction of airborne submicron particulate matter (PM), which is responsible for most of the adverse human health effects, including premature mortality, attributed to poor air quality. Submicron aerosol PM also drives important direct and indirect impacts on atmospheric radiative transfer, causing much of the uncertainty in our understanding of current, and predictions of future, climate change.
Jesse started his mastery of atmospheric organic chemistry as a very productive student in Jim Anderson’s lab at Harvard, focusing on gas phase reaction mechanisms and kinetics of volatile organic compounds with atmospheric oxidants. After a short postdoctoral stint at Harvard he moved on to John Seinfeld’s California Institute of Technology (Caltech) laboratory, where he played a major role in developing and utilizing advanced environmental chambers and a wide range of analytical instrumentation to determine mechanisms and yields of secondary organic aerosol (SOA) particle formation, simulating a range of atmospheric conditions for the photooxidation and condensation of a wide variety of organic vapor precursors.
After three years at Caltech, Jesse returned to the Boston area, joining Aerodyne Research, Inc. (ARI), where he played a leading role in groundbreaking collaborative laboratory measurements using a range of specialized environmental chambers and flow reactors combined with advanced aerosol mass spectrometers and other instruments that better defined the oxidation kinetics and SOA yields for a wide variety of individual organic compounds as well as complex emission sources. This work involved collaborative experiments with colleagues at Harvard University, Boston College, Colorado State University, Lawrence Berkeley National Laboratory, Carnegie Mellon University, and the University of Helsinki.
Since moving on to the Massachusetts Institute of Technology (MIT) in 2009, Jesse has continued many of the collaborations initiated at ARI and established important new ones. He has continued designing and performing a wide range of laboratory and field experiments, many focused on understanding and quantifying the heterogeneous mechanisms and kinetics of SOA particle oxidative aging. He is also engaged in important instrument development work, including the design and field use of a novel method to quantify gas phase emissions of low-volatility organic molecules that are powerful SOA precursors but avoid detection by current gas phase organics monitoring methods. He has also worked with MIT engineers and ARI scientists to develop and utilize advanced aerosol mass spectrometric techniques to better quantify the soot and primary organic aerosol emissions from automotive and aircraft engines.
Just 10 years past his Ph.D., Jesse has an amazing publication record, including 66 archival papers with a collective citation count over 4000, a dozen cited 100 times or more. Several of these papers are fast becoming classics; I anticipate that many of Jesse’s future papers will as well. His Macelwane Medal recognizes extraordinary early career achievements that I expect will be eclipsed by Jesse’s future discoveries.
—CHARLES KOLB, Aerodyne Research, Inc., Billerica, Mass.
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